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WO2008136264A1 - Catalyseur sur support pour réaction d'hydrogénation/déshydrogénation, procédé de fabrication du catalyseur et procédé de stockage/alimentation en hydrogène utilisant ledit catalyseur - Google Patents

Catalyseur sur support pour réaction d'hydrogénation/déshydrogénation, procédé de fabrication du catalyseur et procédé de stockage/alimentation en hydrogène utilisant ledit catalyseur Download PDF

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Publication number
WO2008136264A1
WO2008136264A1 PCT/JP2008/057413 JP2008057413W WO2008136264A1 WO 2008136264 A1 WO2008136264 A1 WO 2008136264A1 JP 2008057413 W JP2008057413 W JP 2008057413W WO 2008136264 A1 WO2008136264 A1 WO 2008136264A1
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WO
WIPO (PCT)
Prior art keywords
catalyst
hydrogenation
production
dehydrogenation reaction
hydrogen storage
Prior art date
Application number
PCT/JP2008/057413
Other languages
English (en)
Japanese (ja)
Inventor
Masaru Ichikawa
Masashi Sakuramoto
Makoto Kurosawa
Satoru Kikuchi
Yukimitsu Mita
Yuji Isaka
Original Assignee
Hrein Energy, Inc.
Alumi Surface Technologies Co., Ltd.
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Hrein Energy, Inc., Alumi Surface Technologies Co., Ltd. filed Critical Hrein Energy, Inc.
Priority to CN200880022491A priority Critical patent/CN101801841A/zh
Publication of WO2008136264A1 publication Critical patent/WO2008136264A1/fr

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    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/22—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by decomposition of gaseous or liquid organic compounds
    • C01B3/24—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by decomposition of gaseous or liquid organic compounds of hydrocarbons
    • C01B3/26—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by decomposition of gaseous or liquid organic compounds of hydrocarbons using catalysts
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
    • B01J23/38—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of noble metals
    • B01J23/40—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of noble metals of the platinum group metals
    • B01J23/42—Platinum
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
    • B01J23/38—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of noble metals
    • B01J23/54—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of noble metals combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36
    • B01J23/56—Platinum group metals
    • B01J23/64—Platinum group metals with arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
    • B01J23/652—Chromium, molybdenum or tungsten
    • B01J23/6525—Molybdenum
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J27/00—Catalysts comprising the elements or compounds of halogens, sulfur, selenium, tellurium, phosphorus or nitrogen; Catalysts comprising carbon compounds
    • B01J27/20—Carbon compounds
    • B01J27/22—Carbides
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J29/00—Catalysts comprising molecular sieves
    • B01J29/03—Catalysts comprising molecular sieves not having base-exchange properties
    • B01J29/0308—Mesoporous materials not having base exchange properties, e.g. Si-MCM-41
    • B01J29/0341—Mesoporous materials not having base exchange properties, e.g. Si-MCM-41 containing arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/0201—Impregnation
    • B01J37/0205—Impregnation in several steps
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/0215—Coating
    • B01J37/0225—Coating of metal substrates
    • B01J37/0226—Oxidation of the substrate, e.g. anodisation
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/16—Reducing
    • B01J37/18—Reducing with gases containing free hydrogen
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C15/00—Cyclic hydrocarbons containing only six-membered aromatic rings as cyclic parts
    • C07C15/02—Monocyclic hydrocarbons
    • C07C15/06—Toluene
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C5/00—Preparation of hydrocarbons from hydrocarbons containing the same number of carbon atoms
    • C07C5/32—Preparation of hydrocarbons from hydrocarbons containing the same number of carbon atoms by dehydrogenation with formation of free hydrogen
    • C07C5/367—Formation of an aromatic six-membered ring from an existing six-membered ring, e.g. dehydrogenation of ethylcyclohexane to ethylbenzene
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J21/00—Catalysts comprising the elements, oxides, or hydroxides of magnesium, boron, aluminium, carbon, silicon, titanium, zirconium, or hafnium
    • B01J21/02—Boron or aluminium; Oxides or hydroxides thereof
    • B01J21/04—Alumina
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J21/00—Catalysts comprising the elements, oxides, or hydroxides of magnesium, boron, aluminium, carbon, silicon, titanium, zirconium, or hafnium
    • B01J21/06—Silicon, titanium, zirconium or hafnium; Oxides or hydroxides thereof
    • B01J21/08—Silica
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J21/00—Catalysts comprising the elements, oxides, or hydroxides of magnesium, boron, aluminium, carbon, silicon, titanium, zirconium, or hafnium
    • B01J21/18—Carbon
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/0201—Impregnation
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/08—Heat treatment
    • B01J37/082—Decomposition and pyrolysis
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/02—Processes for making hydrogen or synthesis gas
    • C01B2203/0266—Processes for making hydrogen or synthesis gas containing a decomposition step
    • C01B2203/0277—Processes for making hydrogen or synthesis gas containing a decomposition step containing a catalytic decomposition step
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/10—Catalysts for performing the hydrogen forming reactions
    • C01B2203/1041—Composition of the catalyst
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/10—Catalysts for performing the hydrogen forming reactions
    • C01B2203/1041—Composition of the catalyst
    • C01B2203/1047—Group VIII metal catalysts
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/10—Catalysts for performing the hydrogen forming reactions
    • C01B2203/1041—Composition of the catalyst
    • C01B2203/1082—Composition of support materials
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/12—Feeding the process for making hydrogen or synthesis gas
    • C01B2203/1205—Composition of the feed
    • C01B2203/1211—Organic compounds or organic mixtures used in the process for making hydrogen or synthesis gas
    • C01B2203/1235—Hydrocarbons
    • C01B2203/1252—Cyclic or aromatic hydrocarbons
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P20/00—Technologies relating to chemical industry
    • Y02P20/50—Improvements relating to the production of bulk chemicals
    • Y02P20/52—Improvements relating to the production of bulk chemicals using catalysts, e.g. selective catalysts

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Materials Engineering (AREA)
  • Inorganic Chemistry (AREA)
  • General Health & Medical Sciences (AREA)
  • Combustion & Propulsion (AREA)
  • Health & Medical Sciences (AREA)
  • Dispersion Chemistry (AREA)
  • Catalysts (AREA)
  • Hydrogen, Water And Hydrids (AREA)
  • Low-Molecular Organic Synthesis Reactions Using Catalysts (AREA)
  • Production Of Liquid Hydrocarbon Mixture For Refining Petroleum (AREA)
  • Fuel Cell (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Abstract

L'objet de l'invention est d'augmenter la vitesse de réaction d'une hydrogénation ou d'une déshydrogénation afin de pouvoir utiliser un catalyseur sur une longue durée. La présente invention concerne un procédé de stockage/alimentation en hydrogène. Ledit procédé comprend la mise en œuvre de la réaction d'hydrogénation pour obtenir un composé aromatique, ou de la réaction de déshydrogénation d'un dérivé hydrogéné du composé aromatique, au moyen d'un catalyseur sur support comprenant du platine et du carbure de molybdène ou du carbure de tungstène recouvrant partiellement ou totalement la surface d'un support.
PCT/JP2008/057413 2007-04-27 2008-04-16 Catalyseur sur support pour réaction d'hydrogénation/déshydrogénation, procédé de fabrication du catalyseur et procédé de stockage/alimentation en hydrogène utilisant ledit catalyseur WO2008136264A1 (fr)

Priority Applications (1)

Application Number Priority Date Filing Date Title
CN200880022491A CN101801841A (zh) 2007-04-27 2008-04-16 氢化/脱氢化反应用载体催化剂、其制备方法以及使用该催化剂的氢储存/供给方法

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP2007118578A JP5122178B2 (ja) 2007-04-27 2007-04-27 水素化／脱水素化反応用担持触媒、その製造方法、およびその触媒を用いた水素貯蔵／供給方法
JP2007-118578 2007-04-27

Publications (1)

Publication Number Publication Date
WO2008136264A1 true WO2008136264A1 (fr) 2008-11-13

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PCT/JP2008/057413 WO2008136264A1 (fr) 2007-04-27 2008-04-16 Catalyseur sur support pour réaction d'hydrogénation/déshydrogénation, procédé de fabrication du catalyseur et procédé de stockage/alimentation en hydrogène utilisant ledit catalyseur

Country Status (3)

Country Link
JP (1) JP5122178B2 (fr)
CN (1) CN101801841A (fr)
WO (1) WO2008136264A1 (fr)

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US9466843B2 (en) 2010-07-30 2016-10-11 Samsung Electronics Co., Ltd. Electrode catalyst and method of preparing electrode catalyst for fuel cell, and membrane electrode assembly and fuel cell including same
CN115485063A (zh) * 2020-04-23 2022-12-16 千代田化工建设株式会社 蛋壳型载铂氧化铝催化剂、其制备方法及其使用方法

Families Citing this family (14)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP5489508B2 (ja) * 2009-03-31 2014-05-14 日立エーアイシー株式会社 水素触媒部材
JP5489509B2 (ja) * 2009-03-31 2014-05-14 日立エーアイシー株式会社 水素触媒部材
JP5620077B2 (ja) * 2009-06-11 2014-11-05 日立エーアイシー株式会社 水素触媒部材
EP2305376A1 (fr) * 2009-09-23 2011-04-06 Lonza Ltd. Procédé et catalyseur pour l'hydrogénation catalytique de composés de nitro aromatiques et hétéro-aromatiques
KR20120115559A (ko) * 2010-02-05 2012-10-18 바스프 에스이 촉매의 제조 방법 및 촉매
JP5369126B2 (ja) * 2010-04-28 2013-12-18 日本精線株式会社 水素化反応／脱水素化反応用のワイヤー触媒成形品
WO2012106349A2 (fr) * 2011-01-31 2012-08-09 The Regents Of The University Of Michigan Catalyseurs haute activité précoces à base de carbure et de nitrure de métal de transition
JP6269297B2 (ja) * 2014-04-25 2018-01-31 トヨタ自動車株式会社 ピストン頂面皮膜方法
CN104307546A (zh) * 2014-11-03 2015-01-28 太仓派欧技术咨询服务有限公司 一种Pt族金属点缀活性点的过渡金属催化剂
CN104307547B (zh) * 2014-11-03 2017-02-15 太仓派欧技术咨询服务有限公司 一种甲烷二氧化碳催化重整反应中的Pt‑ZrO2/WC催化剂
KR102098066B1 (ko) * 2018-04-24 2020-04-07 울산과학기술원 고활성 전극 촉매의 제조방법 및 그를 이용하여 제조된 고활성 전극 촉매
CN111054410B (zh) * 2018-10-16 2023-04-07 中国石油化工股份有限公司 液相脱氢催化剂、制备及用途
CN110124707B (zh) * 2019-06-06 2022-05-31 中山大学 一种螺旋状超低铂载量Mo2C催化剂及其制备方法和应用
FI20235588A1 (en) * 2023-05-26 2024-11-27 North Hydrogen Oy Method and device for the production of hydrogen and the use of a batch of material containing metal

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JP2003117398A (ja) * 2001-10-12 2003-04-22 Toyota Motor Corp Ｗｃ担持触媒及びその製造方法
JP2003334571A (ja) * 2002-03-11 2003-11-25 Nippon Shokubai Co Ltd 排水の処理方法

Patent Citations (2)

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JP2003334571A (ja) * 2002-03-11 2003-11-25 Nippon Shokubai Co Ltd 排水の処理方法

Non-Patent Citations (2)

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LEE S.J. ET AL.: "Preparation and benzene hydrogenation activity of supported molybdenum carbide catalysts", J. CATAL., vol. 128, no. 1, 5 March 1991 (1991-03-05), pages 126 - 136 *
ZELLNER M.B. ET AL.: "Synthesis, characterization and surface reactivity of tungsten carbide (WC) PVD films", SURF. SCI., vol. 569, no. 1-3, 1 August 2004 (2004-08-01), pages 89 - 98, XP004572107, DOI: doi:10.1016/j.susc.2004.07.029 *

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US9466843B2 (en) 2010-07-30 2016-10-11 Samsung Electronics Co., Ltd. Electrode catalyst and method of preparing electrode catalyst for fuel cell, and membrane electrode assembly and fuel cell including same
CN115485063A (zh) * 2020-04-23 2022-12-16 千代田化工建设株式会社 蛋壳型载铂氧化铝催化剂、其制备方法及其使用方法

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Publication number Publication date
CN101801841A (zh) 2010-08-11
JP2008273778A (ja) 2008-11-13
JP5122178B2 (ja) 2013-01-16

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