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WO2018104775A3 - Electrode catalyst for fuel cell, method of producing the same, and fuel cell - Google Patents

Electrode catalyst for fuel cell, method of producing the same, and fuel cell Download PDF

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Publication number
WO2018104775A3
WO2018104775A3 PCT/IB2017/001589 IB2017001589W WO2018104775A3 WO 2018104775 A3 WO2018104775 A3 WO 2018104775A3 IB 2017001589 W IB2017001589 W IB 2017001589W WO 2018104775 A3 WO2018104775 A3 WO 2018104775A3
Authority
WO
WIPO (PCT)
Prior art keywords
fuel cell
carbon support
pores
electrode catalyst
producing
Prior art date
Application number
PCT/IB2017/001589
Other languages
French (fr)
Other versions
WO2018104775A2 (en
Inventor
Nobuaki Mizutani
Yusuke Itoh
Toru Yamamoto
Kotaro HORIAI
Yuki Makino
Mikihiro Kataoka
Original Assignee
Toyota Jidosha Kabushiki Kaisha
Cataler Corporation
Nippon Steel & Sumikin Chemical Co., Ltd.
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Priority claimed from JP2017235057A external-priority patent/JP6969996B2/en
Application filed by Toyota Jidosha Kabushiki Kaisha, Cataler Corporation, Nippon Steel & Sumikin Chemical Co., Ltd. filed Critical Toyota Jidosha Kabushiki Kaisha
Priority to US16/467,677 priority Critical patent/US11258076B2/en
Priority to KR1020197019882A priority patent/KR102239063B1/en
Priority to RU2019121243A priority patent/RU2715385C1/en
Priority to EP17875061.8A priority patent/EP3552261B1/en
Priority to CN201780076163.XA priority patent/CN110383549B/en
Priority to BR112019011531-5A priority patent/BR112019011531B1/en
Publication of WO2018104775A2 publication Critical patent/WO2018104775A2/en
Publication of WO2018104775A3 publication Critical patent/WO2018104775A3/en

Links

Classifications

    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90Selection of catalytic material
    • H01M4/92Metals of platinum group
    • H01M4/925Metals of platinum group supported on carriers, e.g. powder carriers
    • H01M4/926Metals of platinum group supported on carriers, e.g. powder carriers on carbon or graphite
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8803Supports for the deposition of the catalytic active composition
    • H01M4/8807Gas diffusion layers
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8817Treatment of supports before application of the catalytic active composition
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8825Methods for deposition of the catalytic active composition
    • H01M4/8842Coating using a catalyst salt precursor in solution followed by evaporation and reduction of the precursor
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/86Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88Processes of manufacture
    • H01M4/8878Treatment steps after deposition of the catalytic active composition or after shaping of the electrode being free-standing body
    • H01M4/8882Heat treatment, e.g. drying, baking
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M2008/1095Fuel cells with polymeric electrolytes
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30Hydrogen technology
    • Y02E60/50Fuel cells

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Manufacturing & Machinery (AREA)
  • Physics & Mathematics (AREA)
  • Thermal Sciences (AREA)
  • Composite Materials (AREA)
  • Materials Engineering (AREA)
  • Inert Electrodes (AREA)
  • Catalysts (AREA)

Abstract

The present invention relates to an electrode catalyst for a fuel cell that includes a carbon support (11) having pores (13) and catalyst particles containing platinum or a platinum alloy supported on the carbon support (11). The pores (13) of the carbon support (11) have a mode size of pores (13) in a range of 2.1 nm to 5.1 nm. A total pore volume of the pores (13) of the carbon support (11) is in a range of 21 cm3/g to 35 cm3/g. A distance between the catalyst particles and a surface of the carbon support (11) is in a range of 2.0 nm to 12 nm as a distance of a 50% cumulative frequency.
PCT/IB2017/001589 2016-12-09 2017-12-11 Electrode catalyst for fuel cell, method of producing the same, and fuel cell WO2018104775A2 (en)

Priority Applications (6)

Application Number Priority Date Filing Date Title
US16/467,677 US11258076B2 (en) 2016-12-09 2017-12-11 Electrode catalyst for fuel cell, method of producing the same, and fuel cell
KR1020197019882A KR102239063B1 (en) 2016-12-09 2017-12-11 Electrode catalyst for fuel cell, method for manufacturing same, and fuel cell
RU2019121243A RU2715385C1 (en) 2016-12-09 2017-12-11 Electrode catalyst for fuel cells, method of its production and fuel element
EP17875061.8A EP3552261B1 (en) 2016-12-09 2017-12-11 Electrode catalyst for fuel cell, method of producing the same, and fuel cell
CN201780076163.XA CN110383549B (en) 2016-12-09 2017-12-11 Electrode catalyst for fuel cell, method for producing the same, and fuel cell
BR112019011531-5A BR112019011531B1 (en) 2016-12-09 2017-12-11 ELECTRODE CATALYST FOR FUEL CELL, METHOD OF PRODUCING THE SAME AND FUEL CELL

Applications Claiming Priority (4)

Application Number Priority Date Filing Date Title
JP2016-239233 2016-12-09
JP2016239233 2016-12-09
JP2017235057A JP6969996B2 (en) 2016-12-09 2017-12-07 Electrode catalyst for fuel cells and its manufacturing method
JP2017-235057 2017-12-07

Publications (2)

Publication Number Publication Date
WO2018104775A2 WO2018104775A2 (en) 2018-06-14
WO2018104775A3 true WO2018104775A3 (en) 2018-09-13

Family

ID=62218007

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/IB2017/001589 WO2018104775A2 (en) 2016-12-09 2017-12-11 Electrode catalyst for fuel cell, method of producing the same, and fuel cell

Country Status (1)

Country Link
WO (1) WO2018104775A2 (en)

Families Citing this family (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP3970220B1 (en) * 2019-05-13 2023-03-22 Nikola Corporation Catalyst layers of membrane-electrode assemblies and methods of making same
CN111342062A (en) * 2019-10-23 2020-06-26 广东道氏云杉氢能科技有限公司 Supported fuel cell catalyst and application thereof
JP7464553B2 (en) * 2021-03-04 2024-04-09 トヨタ自動車株式会社 Electrocatalyst

Citations (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP2990104A1 (en) * 2013-04-25 2016-03-02 Nissan Motor Co., Ltd. Catalyst, method for producing same, and electrode catalyst layer using said catalyst

Family Cites Families (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP4882225B2 (en) 2004-12-02 2012-02-22 大日本印刷株式会社 Water-repellent electrode catalyst layer, catalyst layer transfer sheet and catalyst layer-electrolyte assembly for polymer electrolyte fuel cell
CN101896424B (en) 2007-12-12 2015-05-13 新日铁住金化学株式会社 Metal encapsulated dendritic carbon nanostructure, carbon nanostructure, process for producing metal encapsulated dendritic carbon nanostructure, process for producing carbon nanostructure, and capacitor
WO2014175100A1 (en) 2013-04-25 2014-10-30 日産自動車株式会社 Catalyst, electrode catalyst layer using said catalyst, membrane electrode assembly, and fuel cell
US10096837B2 (en) 2014-03-19 2018-10-09 Nippon Steel & Sumitomo Metal Corporation Supporting carbon material for solid polymer fuel cell and catalyst metal particle-supporting carbon material

Patent Citations (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP2990104A1 (en) * 2013-04-25 2016-03-02 Nissan Motor Co., Ltd. Catalyst, method for producing same, and electrode catalyst layer using said catalyst

Non-Patent Citations (1)

* Cited by examiner, † Cited by third party
Title
PARK YOUNG-CHUL ET AL: "Effects of carbon supports on Pt distribution, ionomer coverage and cathode performance for polymer electrolyte fuel cells", JOURNAL OF POWER SOURCES, vol. 315, 21 March 2016 (2016-03-21), pages 179 - 191, XP029499867, ISSN: 0378-7753, DOI: 10.1016/J.JPOWSOUR.2016.02.091 *

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