WO2003026051A1 - Membrane-electrode assembly, its manufacturing method, and solid polyer fuel cell using the same - Google Patents

Membrane-electrode assembly, its manufacturing method, and solid polyer fuel cell using the same Download PDF

Info

Publication number: WO2003026051A1
Authority: WO; WIPO (PCT)
Prior art keywords: membrane; electrode assembly; fuel cell; gas; polyer
Prior art date: 2001-09-11

Application number

PCT/JP2002/009144

Other languages

English (en)

French (fr)

Inventor

Osamu Nishikawa

Shigeki Nomura

Masanori Nakamura

Toshiya Sugimoto

Original Assignee

Sekisui Chemical Co., Ltd.

Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)

2001-09-11

Filing date

2002-09-09

Publication date

2003-03-27

2002-09-09 Application filed by Sekisui Chemical Co., Ltd. filed Critical Sekisui Chemical Co., Ltd.

2002-09-09 Priority to US10/415,891 priority Critical patent/US20040053113A1/en

2002-09-09 Priority to EP02760815A priority patent/EP1427043B1/en

2002-09-09 Priority to JP2003529561A priority patent/JP4009593B2/ja

2002-09-09 Priority to KR1020037006329A priority patent/KR100773635B1/ko

2002-09-09 Priority to CA2428131A priority patent/CA2428131C/en

2003-03-27 Publication of WO2003026051A1 publication Critical patent/WO2003026051A1/ja

Links

239000000446 fuel Substances 0.000 title abstract 3
238000004519 manufacturing process Methods 0.000 title abstract 2
239000007787 solid Substances 0.000 title abstract 2
OKKJLVBELUTLKV-UHFFFAOYSA-N Methanol Chemical compound OC OKKJLVBELUTLKV-UHFFFAOYSA-N 0.000 abstract 3
238000009792 diffusion process Methods 0.000 abstract 3
239000012528 membrane Substances 0.000 abstract 3
239000003054 catalyst Substances 0.000 abstract 2
238000004132 cross linking Methods 0.000 abstract 2
229910000510 noble metal Inorganic materials 0.000 abstract 2
OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 abstract 1
229910052760 oxygen Inorganic materials 0.000 abstract 1
239000001301 oxygen Substances 0.000 abstract 1
229920000642 polymer Polymers 0.000 abstract 1
239000000126 substance Substances 0.000 abstract 1

Classifications

- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01B—CABLES; CONDUCTORS; INSULATORS; SELECTION OF MATERIALS FOR THEIR CONDUCTIVE, INSULATING OR DIELECTRIC PROPERTIES
- H01B1/00—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors
- H01B1/06—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors mainly consisting of other non-metallic substances
- H01B1/12—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors mainly consisting of other non-metallic substances organic substances
- H01B1/122—Ionic conductors
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/02—Details
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/02—Details
- H01M8/0297—Arrangements for joining electrodes, reservoir layers, heat exchange units or bipolar separators to each other
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M4/00—Electrodes
- H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
- H01M4/8605—Porous electrodes
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M4/00—Electrodes
- H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
- H01M4/90—Selection of catalytic material
- H01M4/92—Metals of platinum group
- H01M4/925—Metals of platinum group supported on carriers, e.g. powder carriers
- H01M4/926—Metals of platinum group supported on carriers, e.g. powder carriers on carbon or graphite
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/10—Fuel cells with solid electrolytes
- H01M8/1004—Fuel cells with solid electrolytes characterised by membrane-electrode assemblies [MEA]
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/10—Fuel cells with solid electrolytes
- H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
- H01M8/1018—Polymeric electrolyte materials
- H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
- H01M8/1037—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having silicon, e.g. sulfonated crosslinked polydimethylsiloxanes
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/10—Fuel cells with solid electrolytes
- H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
- H01M8/1018—Polymeric electrolyte materials
- H01M8/1041—Polymer electrolyte composites, mixtures or blends
- H01M8/1053—Polymer electrolyte composites, mixtures or blends consisting of layers of polymers with at least one layer being ionically conductive
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/10—Fuel cells with solid electrolytes
- H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
- H01M8/1018—Polymeric electrolyte materials
- H01M8/1069—Polymeric electrolyte materials characterised by the manufacturing processes
- H01M8/1072—Polymeric electrolyte materials characterised by the manufacturing processes by chemical reactions, e.g. in situ polymerisation or in situ crosslinking
- H01M8/1074—Sol-gel processes
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/10—Fuel cells with solid electrolytes
- H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
- H01M8/1018—Polymeric electrolyte materials
- H01M8/1069—Polymeric electrolyte materials characterised by the manufacturing processes
- H01M8/1086—After-treatment of the membrane other than by polymerisation
- H01M8/1088—Chemical modification, e.g. sulfonation
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M2300/00—Electrolytes
- H01M2300/0088—Composites
- H01M2300/0091—Composites in the form of mixtures
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/10—Fuel cells with solid electrolytes
- H01M8/1009—Fuel cells with solid electrolytes with one of the reactants being liquid, solid or liquid-charged
- H01M8/1011—Direct alcohol fuel cells [DAFC], e.g. direct methanol fuel cells [DMFC]
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/30—Hydrogen technology
- Y02E60/50—Fuel cells
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
- Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
- Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

Landscapes

Chemical & Material Sciences (AREA)
General Chemical & Material Sciences (AREA)
Engineering & Computer Science (AREA)
Manufacturing & Machinery (AREA)
Chemical Kinetics & Catalysis (AREA)
Electrochemistry (AREA)
Sustainable Development (AREA)
Life Sciences & Earth Sciences (AREA)
Sustainable Energy (AREA)
Materials Engineering (AREA)
Physics & Mathematics (AREA)
Spectroscopy & Molecular Physics (AREA)
Dispersion Chemistry (AREA)
Crystallography & Structural Chemistry (AREA)
Composite Materials (AREA)
Fuel Cell (AREA)
Inert Electrodes (AREA)

PCT/JP2002/009144 2001-09-11 2002-09-09 Membrane-electrode assembly, its manufacturing method, and solid polyer fuel cell using the same WO2003026051A1 (en)

Priority Applications (5)

Application Number	Priority Date	Filing Date	Title
US10/415,891 US20040053113A1 (en)	2001-09-11	2002-09-09	Membrane-electrode assembly, its manufacturing method, and solid polyer fuel cell using the same
EP02760815A EP1427043B1 (en)	2001-09-11	2002-09-09	Membrane, electrode assembly, its manufacturing method, and solid polyer fuel cell using the same
JP2003529561A JP4009593B2 (ja)	2001-09-11	2002-09-09	膜−電極接合体、その製造方法及びそれを用いた固体高分子形燃料電池
KR1020037006329A KR100773635B1 (ko)	2001-09-11	2002-09-09	막-전극 접합체, 그의 제조 방법 및 이것을 이용한 고체고분자형 연료 전지
CA2428131A CA2428131C (en)	2001-09-11	2002-09-09	Membrane-electrode assembly, method of manufacturing the same, and polymer electrolyte fuel cell using the same

Applications Claiming Priority (6)

Application Number	Priority Date	Filing Date	Title
JP2001275259		2001-09-11
JP2001-275259		2001-09-11
JP2001-298030		2001-09-27
JP2001298030		2001-09-27
JP2001303239		2001-09-28
JP2001-303239		2001-09-28

Publications (1)

Publication Number	Publication Date
WO2003026051A1 true WO2003026051A1 (en)	2003-03-27

Family

ID=27347479

Family Applications (1)

Application Number	Title	Priority Date	Filing Date
PCT/JP2002/009144 WO2003026051A1 (en)	2001-09-11	2002-09-09	Membrane-electrode assembly, its manufacturing method, and solid polyer fuel cell using the same

Country Status (7)

Country	Link
US (1)	US20040053113A1 (ja)
EP (1)	EP1427043B1 (ja)
JP (1)	JP4009593B2 (ja)
KR (1)	KR100773635B1 (ja)
CN (1)	CN100428549C (ja)
CA (1)	CA2428131C (ja)
WO (1)	WO2003026051A1 (ja)

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JP2003178770A (ja) *	2002-12-26	2003-06-27	Sekisui Chem Co Ltd	膜−電極接合体、その製造方法及びそれを用いた固体高分子電解質型または直接メタノール型燃料電池
EP1496561A2 (en)	2003-07-11	2005-01-12	Tokuyama Corporation	A laminate useful as a membrane-electrode assembly for fuel cells, production process therefor and a fuel cell provided with the laminate
JP2005026207A (ja) *	2003-03-10	2005-01-27	Sekisui Chem Co Ltd	固体高分子形燃料電池用電極及びその製造方法
JP2005276599A (ja) *	2004-03-24	2005-10-06	Jsr Corp	電解質膜−電極接合体の製造方法
JP2005302365A (ja) *	2004-04-07	2005-10-27	Sony Corp	複合触媒、燃料電池用電極、及び燃料電池
EP1619692A1 (en) *	2003-04-25	2006-01-25	Sekisui Chemical Co., Ltd.	Proton-conductive film, process for producing the same, and fuel cell empolying the proton-conductive film
EP1635413A1 (en) *	2003-06-13	2006-03-15	Sekisui Chemical Co., Ltd.	Proton conductive film, method for producing same, and fuel cell using same
JP2007073310A (ja) *	2005-09-06	2007-03-22	Sekisui Chem Co Ltd	膜−電極接合体の製造方法、膜−電極接合体及び固体高分子形燃料電池
JP2008500171A (ja) *	2004-05-27	2008-01-10	イー・アイ・デュポン・ドウ・ヌムール・アンド・カンパニー	燃料電池触媒のための貴金属成分および炭素を有する酸化物またはオキシ水酸化物を含んでなるゾル−ゲル誘導複合体
JP2008204918A (ja) *	2007-02-22	2008-09-04	Sanyo Electric Co Ltd	燃料電池用電極および燃料電池
WO2008114688A1 (ja)	2007-03-16	2008-09-25	Sekisui Chemical Co., Ltd.	電極バインダ、電極、膜－電極接合体及び固体高分子形燃料電池
WO2008114664A1 (ja)	2007-03-16	2008-09-25	Sekisui Chemical Co., Ltd.	膜－電極接合剤、接合層付きプロトン伝導性膜、膜－電極接合体、固体高分子形燃料電池及び膜－電極接合体の製造方法
JP2008243688A (ja) *	2007-03-28	2008-10-09	Sanyo Electric Co Ltd	燃料電池用電極、燃料電池用電極の作製方法、および燃料電池
WO2009020154A1 (ja) *	2007-08-06	2009-02-12	Bridgestone Corporation	表示媒体用粒子およびそれを用いた情報表示用パネル
JP2011154969A (ja) *	2010-01-28	2011-08-11	Honda Motor Co Ltd	膜−電極構造体の製造方法
WO2011108252A1 (ja) *	2010-03-05	2011-09-09	パナソニック株式会社	燃料電池用カソード電極の製造方法及び燃料電池用カソード電極
US8057960B2 (en)	2009-04-28	2011-11-15	Panasonic Corporation	Electrode for fuel cells and method for manufacturing the same, and fuel cell using the same
JP2018006195A (ja) *	2016-07-05	2018-01-11	本田技研工業株式会社	電解質膜・電極構造体の製造方法

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JP2005149727A (ja) *	2003-11-11	2005-06-09	Nec Tokin Corp	膜電極接合体およびその製造方法ならびにそれを用いたダイレクト型燃料電池
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DE102005038195A1 (de) *	2005-08-12	2007-02-15	Pemeas Gmbh	Verbesserte Membran-Elektrodeneinheiten und Brennstoffzellen mit langer Lebensdauer
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JP5329962B2 (ja)	2005-09-30	2013-10-30	バトル、メモリアル、インスティテュート	固定化ヘテロポリ酸を含む燃料電池構成要素
KR100953617B1 (ko) *	2006-10-26	2010-04-20	삼성에스디아이 주식회사	연료 전지용 전극, 이를 포함하는 연료 전지용 막-전극어셈블리 및 이를 포함하는 연료 전지 시스템
US7910263B2 (en) *	2006-10-26	2011-03-22	Samsung Sdi Co., Ltd.	Electrode including a heteropoly acid additive for fuel cell, membrane-electrode assembly for fuel cell including same, and fuel cell system including the same
CN101611510B (zh) *	2007-03-16	2013-04-24	积水化学工业株式会社	膜-电极粘接剂、带有接合层的质子传导性膜、膜-电极接合体、固体高分子型燃料电池以及膜-电极接合体的制造方法
JP2008269902A (ja) *	2007-04-19	2008-11-06	Hitachi Ltd	膜／電極接合体及び直接メタノール型燃料電池
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WO2009108222A2 (en) *	2007-11-09	2009-09-03	3M Innovative Properties Company	Polymer electrolytes including heteropolyacids
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- 2002-09-09 JP JP2003529561A patent/JP4009593B2/ja not_active Expired - Fee Related
- 2002-09-09 EP EP02760815A patent/EP1427043B1/en not_active Expired - Lifetime
- 2002-09-09 CA CA2428131A patent/CA2428131C/en not_active Expired - Lifetime
- 2002-09-09 US US10/415,891 patent/US20040053113A1/en not_active Abandoned
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JP2008500171A (ja) *	2004-05-27	2008-01-10	イー・アイ・デュポン・ドウ・ヌムール・アンド・カンパニー	燃料電池触媒のための貴金属成分および炭素を有する酸化物またはオキシ水酸化物を含んでなるゾル−ゲル誘導複合体
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Publication number	Publication date
US20040053113A1 (en)	2004-03-18
EP1427043A4 (en)	2007-10-17
JP4009593B2 (ja)	2007-11-14
KR100773635B1 (ko)	2007-11-05
KR20040029955A (ko)	2004-04-08
CA2428131C (en)	2010-11-16
CN1537340A (zh)	2004-10-13
JPWO2003026051A1 (ja)	2005-01-06
EP1427043A1 (en)	2004-06-09
EP1427043B1 (en)	2011-12-14
CA2428131A1 (en)	2003-03-27
CN100428549C (zh)	2008-10-22

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