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WO2001087992A3 - Kovalent und ionisch vernetzte polymere und polymermembranen - Google Patents

Kovalent und ionisch vernetzte polymere und polymermembranen Download PDF

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Publication number
WO2001087992A3
WO2001087992A3 PCT/EP2001/005644 EP0105644W WO0187992A3 WO 2001087992 A3 WO2001087992 A3 WO 2001087992A3 EP 0105644 W EP0105644 W EP 0105644W WO 0187992 A3 WO0187992 A3 WO 0187992A3
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Prior art keywords
general formula
radical
ionically
partially
polymer membranes
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PCT/EP2001/005644
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English (en)
French (fr)
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WO2001087992A2 (de
Inventor
Jochen Kerres
Wei Zhang
Chy-Ming Tang
Original Assignee
Univ Stuttgart Inst Fuer Chemi
Jochen Kerres
Wei Zhang
Tang Chy Ming
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Univ Stuttgart Inst Fuer Chemi, Jochen Kerres, Wei Zhang, Tang Chy Ming filed Critical Univ Stuttgart Inst Fuer Chemi
Priority to US10/275,854 priority Critical patent/US6767585B2/en
Priority to JP2001585209A priority patent/JP2003533560A/ja
Priority to AU2001281776A priority patent/AU2001281776A1/en
Priority to EP01960223A priority patent/EP1292632A2/de
Priority to BR0110876-0A priority patent/BR0110876A/pt
Priority to CA002407250A priority patent/CA2407250C/en
Publication of WO2001087992A2 publication Critical patent/WO2001087992A2/de
Publication of WO2001087992A3 publication Critical patent/WO2001087992A3/de

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    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G75/00—Macromolecular compounds obtained by reactions forming a linkage containing sulfur with or without nitrogen, oxygen, or carbon in the main chain of the macromolecule
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1032—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having sulfur, e.g. sulfonated-polyethersulfones [S-PES]
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D53/00—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
    • B01D53/22—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols by diffusion
    • B01D53/228—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols by diffusion characterised by specific membranes
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D69/00—Semi-permeable membranes for separation processes or apparatus characterised by their form, structure or properties; Manufacturing processes specially adapted therefor
    • B01D69/02—Semi-permeable membranes for separation processes or apparatus characterised by their form, structure or properties; Manufacturing processes specially adapted therefor characterised by their properties
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G65/00—Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule
    • C08G65/34—Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule from hydroxy compounds or their metallic derivatives
    • C08G65/38—Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule from hydroxy compounds or their metallic derivatives derived from phenols
    • C08G65/40—Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule from hydroxy compounds or their metallic derivatives derived from phenols from phenols (I) and other compounds (II), e.g. OH-Ar-OH + X-Ar-X, where X is halogen atom, i.e. leaving group
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G75/00—Macromolecular compounds obtained by reactions forming a linkage containing sulfur with or without nitrogen, oxygen, or carbon in the main chain of the macromolecule
    • C08G75/20—Polysulfones
    • C08G75/23—Polyethersulfones
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J3/00—Processes of treating or compounding macromolecular substances
    • C08J3/24—Crosslinking, e.g. vulcanising, of macromolecules
    • C08J3/243—Two or more independent types of crosslinking for one or more polymers
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J3/00—Processes of treating or compounding macromolecular substances
    • C08J3/24—Crosslinking, e.g. vulcanising, of macromolecules
    • C08J3/246—Intercrosslinking of at least two polymers
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C08J5/2206—Films, membranes or diaphragms based on organic and/or inorganic macromolecular compounds
    • C08J5/2218—Synthetic macromolecular compounds
    • C08J5/2256—Synthetic macromolecular compounds based on macromolecular compounds obtained by reactions other than those involving carbon-to-carbon bonds, e.g. obtained by polycondensation
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L71/00—Compositions of polyethers obtained by reactions forming an ether link in the main chain; Compositions of derivatives of such polymers
    • C08L71/08—Polyethers derived from hydroxy compounds or from their metallic derivatives
    • C08L71/10—Polyethers derived from hydroxy compounds or from their metallic derivatives from phenols
    • C08L71/12—Polyphenylene oxides
    • C08L71/126—Polyphenylene oxides modified by chemical after-treatment
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/103—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having nitrogen, e.g. sulfonated polybenzimidazoles [S-PBI], polybenzimidazoles with phosphoric acid, sulfonated polyamides [S-PA] or sulfonated polyphosphazenes [S-PPh]
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D2325/00—Details relating to properties of membranes
    • B01D2325/14—Membrane materials having negatively charged functional groups
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D2325/00—Details relating to properties of membranes
    • B01D2325/42—Ion-exchange membranes
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D61/00—Processes of separation using semi-permeable membranes, e.g. dialysis, osmosis or ultrafiltration; Apparatus, accessories or auxiliary operations specially adapted therefor
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2371/00—Characterised by the use of polyethers obtained by reactions forming an ether link in the main chain; Derivatives of such polymers
    • C08J2371/08—Polyethers derived from hydroxy compounds or from their metallic derivatives
    • C08J2371/10—Polyethers derived from hydroxy compounds or from their metallic derivatives from phenols
    • C08J2371/12—Polyphenylene oxides
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2481/00—Characterised by the use of macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing sulfur with or without nitrogen, oxygen, or carbon only; Polysulfones; Derivatives of such polymers
    • C08J2481/06—Polysulfones; Polyethersulfones
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M2008/1095—Fuel cells with polymeric electrolytes
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells

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  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Organic Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • General Chemical & Material Sciences (AREA)
  • Sustainable Energy (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Sustainable Development (AREA)
  • Electrochemistry (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Analytical Chemistry (AREA)
  • Materials Engineering (AREA)
  • Inorganic Chemistry (AREA)
  • Polymers With Sulfur, Phosphorus Or Metals In The Main Chain (AREA)
  • Conductive Materials (AREA)
  • Polyethers (AREA)
  • Other Resins Obtained By Reactions Not Involving Carbon-To-Carbon Unsaturated Bonds (AREA)
  • Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
  • Manufacture Of Macromolecular Shaped Articles (AREA)
  • Fuel Cell (AREA)
  • Separation Using Semi-Permeable Membranes (AREA)

Abstract

Die verliegende Erfindung betrifft kovalent und ionisch vernetzte Polymere aufweisend wiederkehrende Einheiten der allgemeinen Formel (Formula 1), (1) worin Q eine Bindung, Sauerstoff, Schwefel, (Formula 2) oder (2) (Formula 3) ist und (3) der Rest R ein zweiwertiger Rest einer aromatischen oder heteroaromatischen Verbindung ist, welche sich dadurch auszeichnen, dass a) der Rest R zumindest teilweise Substituenten der allgemeinen Formel (4A), (4B), (4C),(4D), (4E), (4F), (4G) und/oder (4H) aufweist, (Formula)(4A) (Formula)(4B) (Formula)(4C) (Formula)(4D) (Formula) (4E). (Formula)(4F) (Formula) (4G) (Formula)(4H) b) der Rest R zumindest teilweise Substituenten der allgemeinen Formel (5A) und/oder (5B) aufweist, (Formula)(5A) (Formula) (5B) und/oder der Rest R zumindest teiweise eine Gruppe der allgemeinen Formel (5C) und/oder (5D) ist (Formula)(5A) (Formula)(5B) und c) der Rest R zumindest teilweise Brücken der allgemeinen Formel (6) aufweist, (Formula) (6) die mindestens zwei Reste R miteinander verbinden, wobei R?1,R2,R3,R4 und R5¿, M,X,Y,Z und m die in der Beschreibung wiedergegebene Bedeutung haben.
PCT/EP2001/005644 2000-05-19 2001-05-17 Kovalent und ionisch vernetzte polymere und polymermembranen WO2001087992A2 (de)

Priority Applications (6)

Application Number Priority Date Filing Date Title
US10/275,854 US6767585B2 (en) 2000-05-19 2001-05-17 Ionically and covalently cross-linked polymers and polymer membranes
JP2001585209A JP2003533560A (ja) 2000-05-19 2001-05-17 共有結合性およびイオン結合性架橋高分子および高分子膜
AU2001281776A AU2001281776A1 (en) 2000-05-19 2001-05-17 Ionically and covalently cross-linked polymers and polymer membranes
EP01960223A EP1292632A2 (de) 2000-05-19 2001-05-17 Kovalent und ionisch vernetzte polymere und polymermembranen
BR0110876-0A BR0110876A (pt) 2000-05-19 2001-05-17 Polìmeros reticulado covalentemente e ionicamente e membranas de polìmeros
CA002407250A CA2407250C (en) 2000-05-19 2001-05-17 Covalently and ionically cross-linked polymers and polymer membranes

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
DE10024576A DE10024576A1 (de) 2000-05-19 2000-05-19 Kovalent und ionisch vernetzte Polymere und Polymermembranen
DE10024576.5 2000-05-19

Publications (2)

Publication Number Publication Date
WO2001087992A2 WO2001087992A2 (de) 2001-11-22
WO2001087992A3 true WO2001087992A3 (de) 2002-05-23

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Country Status (11)

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US (1) US6767585B2 (de)
EP (1) EP1292632A2 (de)
JP (3) JP2003533560A (de)
KR (1) KR20030007583A (de)
CN (1) CN1433442A (de)
AU (1) AU2001281776A1 (de)
BR (1) BR0110876A (de)
CA (1) CA2407250C (de)
DE (1) DE10024576A1 (de)
MY (1) MY128567A (de)
WO (1) WO2001087992A2 (de)

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KR20170036820A (ko) 2012-07-24 2017-04-03 미쯔비시 레이온 가부시끼가이샤 도전체, 도전성 조성물, 및 적층체
WO2014178744A1 (en) * 2013-04-29 2014-11-06 Obschestvo S Ogranichennoi Otvetstvennostyu "Lukoil - Nizhegorodsky Nauchno-Issledovatelsky I Proektny Institut Po Pererabotke Nefti" Fuel cell for generating electricity using hydrogen sulfide as fuel, method for generating electricity and method of purifying hydrogen sulfide-containing gas using the fuel cell
TWI545156B (zh) 2013-05-16 2016-08-11 三菱麗陽股份有限公司 導電性組成物、導電體、積層體及其製造方法、導電性膜及固體電解電容器
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WO2000066254A1 (de) * 1999-04-30 2000-11-09 Universität Stuttgart Stufenweise alkylierung von polymeren aminen
WO2001064773A1 (de) * 2000-03-02 2001-09-07 Celanese Ventures Gmbh Verfahren zur nitrierung und aminierung von arylpolymer
WO2001084657A2 (de) * 2000-05-02 2001-11-08 HÄRING, Rima Polymere membranen

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EP1292632A2 (de) 2003-03-19
US6767585B2 (en) 2004-07-27
DE10024576A1 (de) 2001-11-22
JP2003533560A (ja) 2003-11-11
JP2012111950A (ja) 2012-06-14
WO2001087992A2 (de) 2001-11-22
AU2001281776A1 (en) 2001-11-26
BR0110876A (pt) 2003-03-11
CA2407250A1 (en) 2001-11-22
KR20030007583A (ko) 2003-01-23
MY128567A (en) 2007-02-28
JP2015057484A (ja) 2015-03-26
US20030208014A1 (en) 2003-11-06
JP5661656B2 (ja) 2015-01-28
CN1433442A (zh) 2003-07-30
CA2407250C (en) 2009-09-29

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