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CN115368536A - Mint polyurethane foaming insole with cooling and itching relieving effects and preparation method and application thereof - Google Patents

Mint polyurethane foaming insole with cooling and itching relieving effects and preparation method and application thereof Download PDF

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Publication number
CN115368536A
CN115368536A CN202211066212.0A CN202211066212A CN115368536A CN 115368536 A CN115368536 A CN 115368536A CN 202211066212 A CN202211066212 A CN 202211066212A CN 115368536 A CN115368536 A CN 115368536A
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mint
parts
insole
weight
polyurethane
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CN115368536B (en
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杨伟
李仲颐
杨权
郭金太
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Zulijian Aging Industry Development Co ltd Beijing Branch
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Zulijian Aging Industry Development Co ltd Beijing Branch
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Priority to CN202211066212.0A priority Critical patent/CN115368536B/en
Publication of CN115368536A publication Critical patent/CN115368536A/en
Priority to PCT/CN2023/089998 priority patent/WO2024045650A1/en
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    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00Polymeric products of isocyanates or isothiocyanates
    • C08G18/06Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/70Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
    • C08G18/72Polyisocyanates or polyisothiocyanates
    • C08G18/74Polyisocyanates or polyisothiocyanates cyclic
    • C08G18/76Polyisocyanates or polyisothiocyanates cyclic aromatic
    • C08G18/7657Polyisocyanates or polyisothiocyanates cyclic aromatic containing two or more aromatic rings
    • C08G18/7664Polyisocyanates or polyisothiocyanates cyclic aromatic containing two or more aromatic rings containing alkylene polyphenyl groups
    • C08G18/7671Polyisocyanates or polyisothiocyanates cyclic aromatic containing two or more aromatic rings containing alkylene polyphenyl groups containing only one alkylene bisphenyl group
    • AHUMAN NECESSITIES
    • A43FOOTWEAR
    • A43BCHARACTERISTIC FEATURES OF FOOTWEAR; PARTS OF FOOTWEAR
    • A43B17/00Insoles for insertion, e.g. footbeds or inlays, for attachment to the shoe after the upper has been joined
    • A43B17/08Insoles for insertion, e.g. footbeds or inlays, for attachment to the shoe after the upper has been joined ventilated
    • AHUMAN NECESSITIES
    • A43FOOTWEAR
    • A43BCHARACTERISTIC FEATURES OF FOOTWEAR; PARTS OF FOOTWEAR
    • A43B17/00Insoles for insertion, e.g. footbeds or inlays, for attachment to the shoe after the upper has been joined
    • A43B17/14Insoles for insertion, e.g. footbeds or inlays, for attachment to the shoe after the upper has been joined made of sponge, rubber, or plastic materials
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00Polymeric products of isocyanates or isothiocyanates
    • C08G18/06Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40High-molecular-weight compounds
    • C08G18/4009Two or more macromolecular compounds not provided for in one single group of groups C08G18/42 - C08G18/64
    • C08G18/4018Mixtures of compounds of group C08G18/42 with compounds of group C08G18/48
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    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00Polymeric products of isocyanates or isothiocyanates
    • C08G18/06Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40High-molecular-weight compounds
    • C08G18/42Polycondensates having carboxylic or carbonic ester groups in the main chain
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00Polymeric products of isocyanates or isothiocyanates
    • C08G18/06Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40High-molecular-weight compounds
    • C08G18/48Polyethers
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00Polymeric products of isocyanates or isothiocyanates
    • C08G18/06Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/65Low-molecular-weight compounds having active hydrogen with high-molecular-weight compounds having active hydrogen
    • C08G18/66Compounds of groups C08G18/42, C08G18/48, or C08G18/52
    • C08G18/6603Compounds of groups C08G18/42, C08G18/48, or C08G18/52 with compounds of group C08G18/32 or polyamines of C08G18/38
    • C08G18/6607Compounds of groups C08G18/42, C08G18/48, or C08G18/52 with compounds of group C08G18/32 or polyamines of C08G18/38 with compounds of group C08G18/3203
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00Polymeric products of isocyanates or isothiocyanates
    • C08G18/06Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/65Low-molecular-weight compounds having active hydrogen with high-molecular-weight compounds having active hydrogen
    • C08G18/66Compounds of groups C08G18/42, C08G18/48, or C08G18/52
    • C08G18/6603Compounds of groups C08G18/42, C08G18/48, or C08G18/52 with compounds of group C08G18/32 or polyamines of C08G18/38
    • C08G18/6614Compounds of groups C08G18/42, C08G18/48, or C08G18/52 with compounds of group C08G18/32 or polyamines of C08G18/38 with compounds of group C08G18/3225 or C08G18/3271 and/or polyamines of C08G18/38
    • C08G18/6622Compounds of groups C08G18/42, C08G18/48, or C08G18/52 with compounds of group C08G18/32 or polyamines of C08G18/38 with compounds of group C08G18/3225 or C08G18/3271 and/or polyamines of C08G18/38 with compounds of group C08G18/3271
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K5/00Use of organic ingredients
    • C08K5/0008Organic ingredients according to more than one of the "one dot" groups of C08K5/01 - C08K5/59
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    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K7/00Use of ingredients characterised by shape
    • C08K7/22Expanded, porous or hollow particles
    • C08K7/24Expanded, porous or hollow particles inorganic
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L99/00Compositions of natural macromolecular compounds or of derivatives thereof not provided for in groups C08L89/00 - C08L97/00
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G2101/00Manufacture of cellular products
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G2110/00Foam properties
    • C08G2110/0083Foam properties prepared using water as the sole blowing agent
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02ATECHNOLOGIES FOR ADAPTATION TO CLIMATE CHANGE
    • Y02A50/00TECHNOLOGIES FOR ADAPTATION TO CLIMATE CHANGE in human health protection, e.g. against extreme weather
    • Y02A50/30Against vector-borne diseases, e.g. mosquito-borne, fly-borne, tick-borne or waterborne diseases whose impact is exacerbated by climate change

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  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Footwear And Its Accessory, Manufacturing Method And Apparatuses (AREA)

Abstract

The invention provides a mint polyurethane foaming insole with cooling and itching relieving effects and a preparation method and application thereof, wherein the preparation raw materials of the mint polyurethane foaming insole comprise a combination of polymer polyol, diisocyanate, a foaming agent, activated carbon, a chain extender, mint oil and mint powder in a specific part; the mint polyurethane foaming insole is prepared by adding the mint oil, the mint powder and the active carbon into the preparation raw materials for matching, coordination and synergism are achieved, so that the finally prepared mint polyurethane foaming insole has lasting and excellent cooling and itching relieving effects, is high in air permeability and wearing comfort, has the effects of absorbing odor, absorbing moisture, removing peculiar smell, preventing mildew and resisting bacteria, and has important research value.

Description

Mint polyurethane foaming insole with cooling and itching relieving effects and preparation method and application thereof
Technical Field
The invention belongs to the technical field of polyurethane insoles, and particularly relates to a mint polyurethane foaming insole with cooling and itching relieving effects and a preparation method and application thereof.
Background
The shoe is an indispensable daily necessity for people to engage in life and work, and the insole is an important component of the shoe, so the importance of the insole directly influences the comfort level of the shoe. The traditional insoles sold in the market at present are generally made of cotton cloth, and although the wearing feeling is comfortable, the phenomena of dampness and foot odor generation caused by the absorption of foot sweat of the cotton insole are quite common, especially the foot which is easy to sweat; meanwhile, bacteria in the shoes are easy to grow and breed due to the humidity, and the feet are greatly influenced; in addition, most insoles are made of plastic or polymer materials, but the pure plastic or polymer materials have poor moisture absorption capability and do not have odor absorption and antibacterial effects, so that the preparation of insoles with the moisture absorption, odor absorption and antibacterial effects is always the focus of research in the field.
CN106388125A discloses a deodorant, antibacterial and healthy Chinese herbal medicine PU insole, which comprises an upper wear-resistant layer, a lower wear-resistant layer and a deodorant and antibacterial layer positioned between the upper wear-resistant layer and the lower wear-resistant layer, wherein the deodorant and antibacterial raw material components comprise polyurethane waste, toner, tea polyphenol, PU elastomer, cork particles and Chinese herbal medicine components consisting of rhubarb, sophora flavescens, peach kernel, mint, borneol, talcum powder and agilawood; the deodorization and antibacterial layer in the Chinese herbal medicine PU insole adopts a PU foam layer, has tens of thousands of ultrafine, open and intercommunicated honeycomb pores, has super-strong moisture absorption, permeation and exhaust capabilities, and can effectively solve the problems of high density, poor moisture absorption and poor air permeability of the traditional EVA insole.
CN112806667A discloses a Chinese hemp Chinese herbal medicine foot-care massage health preserving bacteriostatic insole and a preparation method thereof, wherein an insole body comprises a polyurethane layer, the polyurethane layer has high wear resistance and light weight, an upper linen layer is pressed on the upper surface of the polyurethane layer, a lower linen layer is pressed on the lower surface of the polyurethane layer, the air permeability, the bacteriostatic property and the water absorption of the linen layer are enhanced by a manufacturing process of the linen, and the following raw materials are placed in a cavity of the polyurethane layer: 1-3 g of lavender, 2-3 g of rosemary and 1-3 g of mint; 3-4 g of wormwood; 1-2 g of eucalyptus leaves; 1-2 g of pearl powder; 3-4 g of phellodendron; 3-4 g of radix sophorae flavescentis; 3-4 g of golden larch bark; 2-3 g of basil; 2-3 g of lemon grass, and the traditional Chinese medicines have the effects of tonifying spleen, soothing nerves, clearing away heat and toxic materials, warming and activating meridian, promoting qi and blood circulation, and detoxifying and reducing swelling, so that the insole using the traditional Chinese medicines has the effects of health preserving and health care on a human body.
However, the shoe pad provided by the prior art has poor persistence of the effects of deodorization, bacteriostasis and the like, and the effect is single, and the prepared shoe pad cannot have the effects of ventilation, sweat absorption, deodorization, odor removal, mildew prevention, antibiosis, cooling and itching relief.
Therefore, in order to solve the problems, the mint polyurethane foaming insole which has the effects of ventilation, sweat absorption, deodorization and odor removal and also has the effects of cooling and relieving itching needs to be developed at present.
Disclosure of Invention
Aiming at the defects of the prior art, the invention aims to provide the mint polyurethane foaming insole with the effects of cooling and relieving itching and the preparation method and application thereof.
In order to achieve the purpose, the invention adopts the following technical scheme:
according to the first aspect, the invention provides a mint polyurethane foaming insole with cooling and itching relieving effects, which is prepared from the following raw materials in parts by weight: 40-50 parts of polymer polyol, 25-35 parts of diisocyanate, 2-3 parts of foaming agent, 1-2 parts of activated carbon, 4-6 parts of chain extender, 1-3 parts of peppermint oil and 5-7 parts of peppermint oil.
Wherein the polymer polyol may be 41 parts by weight, 42 parts by weight, 43 parts by weight, 44 parts by weight, 45 parts by weight, 46 parts by weight, 47 parts by weight, 48 parts by weight, 49 parts by weight, or the like.
The diisocyanate may be 26 parts by weight, 27 parts by weight, 28 parts by weight, 29 parts by weight, 30 parts by weight, 31 parts by weight, 32 parts by weight, 33 parts by weight, 34 parts by weight, or the like.
The blowing agent may be 2.1 parts by weight, 2.2 parts by weight, 2.3 parts by weight, 2.4 parts by weight, 2.5 parts by weight, 2.6 parts by weight, 2.7 parts by weight, 2.8 parts by weight, 2.9 parts by weight, or the like.
The activated carbon may be 1.1, 1.2, 1.3, 1.4, 1.5, 1.6, 1.7, 1.8, or 1.9 parts by weight, or the like.
The chain extender may be 4.2 parts by weight, 4.4 parts by weight, 4.6 parts by weight, 4.8 parts by weight, 5 parts by weight, 5.2 parts by weight, 5.4 parts by weight, 5.6 parts by weight, or 5.8 parts by weight, and the like.
The peppermint oil may be 1.2 parts by weight, 1.4 parts by weight, 1.6 parts by weight, 1.8 parts by weight, 2 parts by weight, 2.2 parts by weight, 2.4 parts by weight, 2.6 parts by weight, 2.8 parts by weight, or the like.
The mint powder may be 5.2, 5.4, 5.6, 5.8, 6, 6.2, 6.4, 6.6, or 6.8 parts by weight, etc.
The preparation raw materials of the mint polyurethane foaming insole with the cooling and itching relieving effects comprise polymer polyol, diisocyanate, a foaming agent, activated carbon, a chain extender, mint oil and mint powder; on one hand, the mint powder can be adsorbed by the active carbon, so that the mint powder is firmly fixed in the insole, the mint powder is prevented from being rapidly dissipated in the use process of the insole, the mint powder contains a large amount of mint oil, the mint oil can be gradually volatilized, and the mint oil added at the beginning is matched, so that the insole can be ensured to have a lasting and effective cooling and itching relieving effect in the whole use process; on the other hand, the activated carbon, the mint oil and the mint powder are matched together, so that the effects of absorbing odor, absorbing moisture, removing peculiar smell, preventing mildew and resisting bacteria are achieved, and the obtained mint polyurethane foamed insole has excellent sweat absorbing and deodorizing functions, anti-mildew and anti-bacteria functions and wearing comfort.
Preferably, the polymer polyol comprises a polyether polyol and/or a polyester polyol.
Preferably, the diisocyanate comprises diphenylmethane diisocyanate.
Preferably, the blowing agent comprises water.
Preferably, the chain extender comprises a combination of ethylene glycol and diethanolamine.
Preferably, the content of the glycol in the preparation raw material of the mint polyurethane foaming insole is 3 to 4 parts by weight, such as 3.1 parts by weight, 3.2 parts by weight, 3.3 parts by weight, 3.4 parts by weight, 3.5 parts by weight, 3.6 parts by weight, 3.7 parts by weight, 3.8 parts by weight or 3.9 parts by weight, and the like.
Preferably, the content of the diethanol ammonia in the preparation raw materials of the mint polyurethane foaming insole is 1 to 2 parts by weight, such as 1.2 parts by weight, 1.3 parts by weight, 1.4 parts by weight, 1.5 parts by weight, 1.6 parts by weight, 1.7 parts by weight, 1.8 parts by weight or 1.9 parts by weight and the like.
Preferably, the mass ratio of the peppermint oil to the peppermint powder is 1 (2-4), such as 1.
According to the preferred technical scheme, the mass ratio of the mint oil to the mint powder added in the preparation raw materials is limited to 1 (2-4), so that the obtained mint polyurethane foamed insole can exert the cooling and itching relieving effects most excellently and has the most lasting effect. On one hand, if the addition amount of the peppermint oil is too low, the cooling and itching relieving effect at the early stage of the use of the insole is not obvious; on the other hand, if the addition amount of the mint powder is too low, the cooling and itching relieving effect of the insole at the later use stage is not obvious, and the durability in use is poor.
Preferably, the preparation raw materials of the mint polyurethane foaming insole also comprise an antibacterial agent.
Preferably, the antibacterial agent is contained in 0.5-1.5 parts by weight, such as 0.6 part by weight, 0.7 part by weight, 0.8 part by weight, 0.9 part by weight, 1 part by weight, 1.1 part by weight, 1.2 parts by weight, 1.3 parts by weight, 1.4 parts by weight, or the like, in the raw material for preparing the mint polyurethane foamed insole.
Preferably, the preparation raw materials of the mint polyurethane foaming insole also comprise any one or the combination of at least two of silicone oil, color paste or water.
Preferably, the content of the silicone oil in the preparation raw material of the mint polyurethane foam insole is 1 to 3 parts by weight, such as 1.2 parts by weight, 1.4 parts by weight, 1.6 parts by weight, 1.8 parts by weight, 2 parts by weight, 2.2 parts by weight, 2.4 parts by weight, 2.6 parts by weight or 2.8 parts by weight, and the like.
Preferably, the content of the color paste in the preparation raw materials of the mint polyurethane foaming insole is 1 to 2 parts by weight, such as 1.2 parts by weight, 1.3 parts by weight, 1.4 parts by weight, 1.5 parts by weight, 1.6 parts by weight, 1.7 parts by weight, 1.8 parts by weight or 1.9 parts by weight.
Preferably, the content of water in the raw materials for preparing the mint polyurethane foamed insole is 0.5-1.5 parts by weight, such as 0.6 part by weight, 0.7 part by weight, 0.8 part by weight, 0.9 part by weight, 1 part by weight, 1.1 part by weight, 1.2 parts by weight, 1.3 parts by weight or 1.4 parts by weight, and the like.
In a second aspect, the present invention provides a method for preparing a mint polyurethane foam insole, which comprises: mixing polymer polyol, a foaming agent, activated carbon, a chain extender, mint oil, mint powder, optional silicone oil and optional color paste in water, adding isocyanate to react, and performing foaming molding to obtain the mint polyurethane foamed insole.
Preferably, the temperature of the mixing is 70 to 90 ℃, such as 72 ℃, 74 ℃, 76 ℃, 78 ℃, 80 ℃, 82 ℃, 84 ℃, 86 ℃ or 88 ℃, etc.
Preferably, the mixing time is 1-30 min, such as 2min, 4min, 6min, 8min, 10min, 12min, 14min, 16min, 18min, 20min, 22min, 24min, 26min, 28min, and the like.
Preferably, the reaction time is 1 to 2 hours, such as 1.1h, 1.2h, 1.3h, 1.4h, 1.5h, 1.6h, 1.7h, 1.8h, 1.9h, and the like.
Preferably, the reaction temperature is 90-110 ℃, such as 92 ℃, 94 ℃, 96 ℃, 98 ℃, 100 ℃, 102 ℃, 104 ℃, 106 ℃ or 108 ℃.
In a third aspect, the present invention provides a use of a menthe polyurethane foam insole as described in the first aspect in footwear.
Preferably, the shoe comprises a sports shoe.
Compared with the prior art, the invention has the following beneficial effects:
the preparation raw materials of the mint polyurethane foaming insole with the cooling and itching relieving effects comprise polymer polyol, diisocyanate, a foaming agent, activated carbon, a chain extender, mint oil and mint powder; the mint oil, the mint powder and the active carbon in specific parts are added into the preparation raw materials for matching, and the synergistic effect is realized, so that the obtained mint polyurethane foamed insole has a lasting and effective cooling and itching relieving effect, and also has high air permeability and excellent sweat stain resistance color fastness; specifically, the air permeability of the mint polyurethane foamed insole obtained by the invention is 122-135 mm/s, the color fastness to perspiration can reach 3-4 level, and the cool and itching relieving effect test shows that the mint polyurethane foamed insole has a cool effect immediately after the insole is used and after the insole is used for one month, and has higher wearing comfort.
Detailed Description
The technical solution of the present invention is further explained by the following embodiments. It should be understood by those skilled in the art that the examples are only for the understanding of the present invention and should not be construed as the specific limitation of the present invention.
The raw materials and their sources, including manufacturer and model information, referred to in the detailed description of the invention are shown in table 1 below:
TABLE 1
Figure BDA0003827625380000061
Figure BDA0003827625380000071
Example 1
A mint polyurethane foaming insole with cooling and itching relieving effects is prepared from the following raw materials in parts by weight:
Figure BDA0003827625380000072
the preparation method of the mint polyurethane foamed insole provided by the embodiment comprises the following steps: and (2) mixing polyether polyol, polyester polyol, a foaming agent, activated carbon, ethylene glycol, diethanol ammonia, peppermint oil, peppermint powder, silicone oil and color paste in water at the temperature of 80 ℃ for 20min, adding diphenylmethane diisocyanate to react at the temperature of 100 ℃ for 30min, and performing foaming molding in a mold to obtain the peppermint polyurethane foamed insole.
Example 2
A mint polyurethane foaming insole with cooling and itching relieving effects is prepared from the following raw materials in parts by weight:
Figure BDA0003827625380000081
the preparation method of the mint polyurethane foamed insole provided in this example is the same as that of example 1.
Example 3
A mint polyurethane foaming insole with cooling and itching relieving effects is prepared from the following raw materials in parts by weight:
Figure BDA0003827625380000082
Figure BDA0003827625380000091
the preparation method of the mint polyurethane foamed insole provided in this example is the same as that of example 1.
Example 4
A mint polyurethane foaming insole with cooling and itching relieving effects is only different from that in example 1 in that the mint oil is added in an amount of 1 part by weight, the mint powder is added in an amount of 7 parts by weight, and other components, the using amount and the preparation method are the same as those in example 1.
Example 5
A mint polyurethane foaming insole with cooling and itching relieving effects is different from example 1 only in that 3 parts by weight of mint oil and 5 parts by weight of mint powder are added, and other components, the using amount and the preparation method are the same as those of example 1.
Comparative example 1
A polyurethane foam insole which is different from the polyurethane foam insole in example 1 only in that activated carbon is not added, and other components, the amount and the preparation method are the same as those of example 1.
Comparative example 2
A polyurethane foaming insole is different from the polyurethane foaming insole in example 1 only in that mint powder is not added, the addition amount of mint oil is 8 parts by weight, and other components, the use amount and the preparation method are the same as those of example 1.
Comparative example 3
A polyurethane foaming insole is different from the polyurethane foaming insole in example 1 only in that peppermint oil is not added, the addition amount of peppermint powder is 8 parts by weight, and other components, the use amount and the preparation method are the same as those of example 1.
Comparative example 4
A polyurethane foam insole which is different from the polyurethane foam insole in example 1 only in that peppermint oil and peppermint powder are not added, and other components, the using amount and the preparation method are the same as those of example 1.
Comparative example 5
A polyurethane foam insole which is different from the polyurethane foam insole in example 1 only in that peppermint oil, peppermint powder and activated carbon are not added, and other components, the using amount and the preparation method are the same as those of example 1.
And (3) performance testing:
(1) Air permeability: the test was carried out according to the preparation method provided in GB/T5453-1997;
(2) Color fastness to perspiration: testing according to a testing method provided by GB/T3922-2013, and testing the color change grade under an acidic condition;
(3) Cooling and itching relieving effects: 100 volunteers were selected, 20 test subjects per test group, and the use effect was recorded at the beginning of use and after 1 month of use using the polyurethane foam insole provided in examples and comparative examples.
The polyurethane foam insoles provided in examples 1 to 5 and comparative examples 1 to 5 were tested according to the above test method, and the test results are shown in Table 2:
TABLE 2
Figure BDA0003827625380000101
Figure BDA0003827625380000111
As can be seen from the data in table 2:
the mint polyurethane foaming insole provided by the invention has effective air permeability and color fastness to perspiration, and also has lasting and effective cooling and itching relieving effects; specifically, the air permeability of the mint polyurethane foamed insoles obtained in examples 1 to 5 is 122 to 135mm/s, the color fastness to perspiration can reach 3 to 4 grades, and the cool and itching relieving effect test shows that the mint polyurethane foamed insoles have the cool and refreshing effect both at the beginning of the use of the insoles and after one month of the use of the insoles.
Comparing example 1 with comparative example 1, it can be seen that the polyurethane shoe insole obtained without adding activated carbon has reduced air permeability and color fastness to perspiration, and the cooling and itching relieving effect is not felt at all after 1 month of use, indicating that the cooling and itching relieving effect of the polyurethane shoe insole obtained in comparative example 1 is poor in durability.
Comparing example 1 with comparative examples 2 to 3 again, it can be found that the polyurethane insole obtained without adding peppermint powder (comparative example 2) has poor durability of the cooling and itching relieving effect; the polyurethane insole obtained without the addition of peppermint oil (comparative example 3) had a poor initial cooling and itching relieving effect.
Further comparing example 1 with comparative examples 4 to 5, it was found that the polyurethane insole obtained without adding peppermint oil and peppermint powder (comparative example 4) had no cooling and itching relieving effects; the polyurethane insole obtained without adding the peppermint oil, the peppermint powder and the activated carbon (comparative example 5) has no cooling and itching relieving effect and poor air permeability.
Finally, comparing example 1 with examples 4 to 5, it can be seen that the ratio of the mint oil and the mint powder added does not fall within the range defined in the present application, and the cooling, itching relieving effect and the air permeability of the obtained polyurethane insole are also affected.
The applicant states that the invention is described by the above examples as a mint polyurethane foam insole with cooling and itching relieving effects, and a preparation method and application thereof, but the invention is not limited to the above examples, that is, the invention is not limited to the above examples. It should be understood by those skilled in the art that any modification of the present invention, equivalent substitutions of the raw materials of the product of the present invention, addition of auxiliary components, selection of specific modes, etc., are within the scope and disclosure of the present invention.

Claims (10)

1. The mint polyurethane foaming insole with the effects of cooling and relieving itching is characterized by comprising the following raw materials in parts by weight: 40 to 50 parts of polymer polyol, 25 to 35 parts of diisocyanate, 2 to 3 parts of foaming agent, 1 to 2 parts of activated carbon, 4 to 6 parts of chain extender, 1 to 3 parts of peppermint oil and 5 to 7 parts of peppermint powder.
2. The menthane foamed insole of claim 1, wherein the polymer polyol comprises polyether polyol and/or polyester polyol;
preferably, the diisocyanate comprises diphenylmethane diisocyanate.
3. The mentha haplocalyx polyurethane foam insole of claim 1 or 2, wherein the foaming agent comprises water;
preferably, the chain extender comprises a combination of ethylene glycol and diethanolamine;
preferably, the content of ethylene glycol in the preparation raw materials of the mint polyurethane foaming insole is 3-4 parts by weight;
preferably, the content of the diethanol ammonia in the preparation raw materials of the mint polyurethane foaming insole is 1 to 2 parts by weight.
4. The mint polyurethane foam insole according to any one of claims 1 to 3, wherein the weight ratio of the mint oil to the mint powder is 1 (2-4).
5. The mint polyurethane foaming insole according to any one of claims 1 to 4, wherein raw materials for preparing the mint polyurethane foaming insole further comprise an antibacterial agent;
preferably, the antibacterial agent content in the preparation raw materials of the mint polyurethane foaming insole is 0.5-1.5 parts by weight.
6. The mint polyurethane foaming insole according to any one of claims 1 to 5, wherein the mint polyurethane foaming insole is prepared from raw materials which further comprise any one or a combination of at least two of silicone oil, color paste or water;
preferably, the content of silicone oil in the preparation raw materials of the mint polyurethane foaming insole is 1-3 parts by weight;
preferably, the content of the color paste in the preparation raw materials of the mint polyurethane foamed insole is 1 to 2 parts by weight;
preferably, the content of water in the preparation raw materials of the mint polyurethane foaming insole is 0.5-1.5 parts by weight.
7. A method for preparing the mint polyurethane foam insole as claimed in any one of claims 1 to 6, wherein the method comprises the following steps: mixing polymer polyol, a foaming agent, activated carbon, a chain extender, peppermint oil, peppermint powder, optional silicone oil and optional color paste in water, adding diisocyanate for reaction, and performing foaming molding to obtain the peppermint polyurethane foamed insole.
8. The method of claim 7, wherein the temperature of the mixing is 70 to 90 ℃;
preferably, the mixing time is 1 to 30min.
9. The method according to claim 7 or 8, wherein the reaction time is 1 to 2 hours;
preferably, the temperature of the reaction is 90 to 110 ℃.
10. Use of a mentha haplocalyx polyurethane foam insole as claimed in any one of claims 1 to 6 in footwear;
preferably, the shoe comprises a sports shoe.
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