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    Direct Visualization of Laser-Driven Electron Multiple Scattering and Tunneling Distance in Strong-Field Ionization

    Daniel D. Hickstein1, Predrag Ranitovic1,*, Stefan Witte1,2, Xiao-Min Tong3, Ymkje Huismans4, Paul Arpin1, Xibin Zhou1, K. Ellen Keister1, Craig W. Hogle1 et al.

    Bosheng Zhang1, Chengyuan Ding1, Per Johnsson5, N. Toshima3, Marc J. J. Vrakking6, Margaret M. Murnane1, and Henry C. Kapteyn1

    • 1JILA and Department of Physics, University of Colorado at Boulder and NIST, Boulder, Colorado 80303, USA
    • 2Institute for Lasers, Life and Biophotonics, VU University, De Boelelaan 1081, 1081 HV Amsterdam, The Netherlands
    • 3Division of Materials Science, Faculty of Pure and Applied Sciences, University of Tsukuba, Ibaraki 305-8573, Japan
    • 4FOM Institute AMOLF, Science Park 104, 1098 XG Amsterdam, The Netherlands
    • 5Lund University, P. O. Box 118, SE-221 00 Lund, Sweden
    • 6Max-Born-Institute, Max-Born Strasse 2A, D-12489 Berlin, Germany
    • *To whom all correspondence (inquiry) should be addressed. pranitovic@lbl.gov

    Phys. Rev. Lett. 109, 073004 – Published 16 August, 2012

    DOI: https://doi.org/10.1103/PhysRevLett.109.073004

    Abstract

    Using a simple model of strong-field ionization of atoms that generalizes the well-known 3-step model from 1D to 3D, we show that the experimental photoelectron angular distributions resulting from laser ionization of xenon and argon display prominent structures that correspond to electrons that pass by their parent ion more than once before strongly scattering. The shape of these structures can be associated with the specific number of times the electron is driven past its parent ion in the laser field before scattering. Furthermore, a careful analysis of the cutoff energy of the structures allows us to experimentally measure the distance between the electron and ion at the moment of tunnel ionization. This work provides new physical insight into how atoms ionize in strong laser fields and has implications for further efforts to extract atomic and molecular dynamics from strong-field physics.

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