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    Attosecond Probe of Valence-Electron Wave Packets by Subcycle Sculpted Laser Fields

    Xinhua Xie1, Stefan Roither1, Daniil Kartashov1, Emil Persson2, Diego G. Arbó2,3, Li Zhang1, Stefanie Gräfe2, Markus S. Schöffler1, Joachim Burgdörfer2 et al.

    Andrius Baltuška1 and Markus Kitzler1,*

    • 1Photonics Institute, Vienna University of Technology, A-1040 Vienna, Austria, EU
    • 2Institute for Theoretical Physics, Vienna University of Technology, A-1040 Vienna, Austria, EU
    • 3Institute for Astronomy and Space Physics - IAFE (FCEN-UBA Conicet), Buenos Aires, Argentina
    • *Corresponding author. markus.kitzler@tuwien.ac.at

    Phys. Rev. Lett. 108, 193004 – Published 9 May, 2012

    DOI: https://doi.org/10.1103/PhysRevLett.108.193004

    Abstract

    We experimentally and theoretically demonstrate a self-referenced wave-function retrieval of a valence-electron wave packet during its creation by strong-field ionization with a sculpted laser field. Key is the control over interferences arising at different time scales. Our work shows that the measurement of subcycle electron wave-packet interference patterns can serve as a tool to retrieve the structure and dynamics of the valence-electron cloud in atoms on a sub-10-as time scale.

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