Continuum in the Spin-Excitation Spectrum of a Haldane Chain Observed by Neutron Scattering in
Phys. Rev. Lett. 87, 017202 – Published 15 June, 2001Erratum Phys. Rev. Lett. 91, 039902 (2003)
DOI: https://doi.org/10.1103/PhysRevLett.87.017202
Abstract
The spin-excitation continuum, expected to dominate the low-energy fluctuation spectrum in the Haldane spin chain around the Brillouin zone center, , is directly observed by inelastic magnetic neutron scattering in the quasi-1D antiferromagnet . We find that the single mode approximation fails, and that a finite energy width appears in the dynamic correlation function for . The width increases with decreasing , while acquires an asymmetric shape qualitatively similar to that predicted for the two-magnon continuum in the nonlinear -model.