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    Continuum in the Spin-Excitation Spectrum of a Haldane Chain Observed by Neutron Scattering in CsNiCl3

    I. A. Zaliznyak1, S.-H. Lee2,3, and S. V. Petrov4

    • 1Department of Physics, Brookhaven National Laboratory, Upton, New York 11973-5000
    • 2National Institute of Standards and Technology, Gaithersburg, Maryland 20899
    • 3Department of Physics, University of Maryland, College Park, Maryland 20742
    • 4P. Kapitza Institute for Physical Problems, ulica Kosygina, 2, Moscow, 117334 Russia

    Phys. Rev. Lett. 87, 017202 – Published 15 June, 2001Erratum Phys. Rev. Lett. 91, 039902 (2003)

    DOI: https://doi.org/10.1103/PhysRevLett.87.017202

    Abstract

    The spin-excitation continuum, expected to dominate the low-energy fluctuation spectrum in the Haldane spin chain around the Brillouin zone center, q=0, is directly observed by inelastic magnetic neutron scattering in the S=1 quasi-1D antiferromagnet CsNiCl3. We find that the single mode approximation fails, and that a finite energy width appears in the dynamic correlation function S(q,ω) for q0.5π. The width increases with decreasing q, while S(q,ω) acquires an asymmetric shape qualitatively similar to that predicted for the two-magnon continuum in the nonlinear σ-model.

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