Evolution of spin excitations in a gapped antiferromagnet from the quantum to the high-temperature limit
Phys. Rev. B 66, 174412 – Published 8 November, 2002
DOI: https://doi.org/10.1103/PhysRevB.66.174412
Abstract
We have mapped from the quantum to the classical limit the spin excitation spectrum of the antiferromagnetic spin-1 Heisenberg chain system in its paramagnetic phase from to Neutron scattering shows that the excitations are resonant and dispersive up to at least but broaden considerably with increasing temperature. The dispersion flattens out with increasing temperature as the resonance energy at the antiferromagnetic wave vector increases and the maximum in the dispersion decreases. The correlation length between and is in agreement with quantum Monte Carlo calculations for the spin-1 chain. is also consistent with the single mode approximation, suggesting that the excitations are short-lived single particle excitations. Below where three-dimensional spin correlations are important, is shorter than predicted and the experiment is not consistent with the random phase approximation for coupled quantum chains. At the structure factor and second energy moment of the excitation spectrum are in excellent agreement with the high-temperature series expansion.